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SLAC Publication: SLAC-PUB-15824
SLAC Release Date: November 1, 2013
Examining Electron-boson Coupling using Time-resolved Spectroscopy
Sentef, Michael.
Nonequilibrium pump-probe time domain spectroscopies can become an important tool to disentangle degrees of freedom whose coupling leads to broad structures in the frequency domain. Here, using the time-resolved solution of a model photoexcited electron-phonon system we show that the relaxational dynamics are directly governed by the equilibrium self-energy so that the phonon frequency sets a window for slow versus fast recovery. The overall temporal structure of this relaxation spectroscopy all... Show Full Abstract
Nonequilibrium pump-probe time domain spectroscopies can become an important tool to disentangle degrees of freedom whose coupling leads to broad structures in the frequency domain. Here, using the time-resolved solution of a model photoexcited electron-phonon system we show that the relaxational dynamics are directly governed by the equilibrium self-energy so that the phonon frequency sets a window for slow versus fast recovery. The overall temporal structure of this relaxation spectroscopy allows for a reliable and quantitative extraction of the electron-phonon coupling strength without requiring an effective temperature model or making strong assumptions about the underlying bare electronic band dispersion. Show Partial Abstract
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  • Interest Categories: Material Sciences